The use of TiO2 as catalyst in thin film fixed bed reactor for the treatment of landfill water

Authors

  • Redha Kernani Department of Chemistry,University of Bejaia,Tharga Ouzemour Road, Bejaia, 06000. Algeria
  • Nabil Mameri Ecole Nationale Polytechnique, Unité URIE, 10 Avenue Pasteur, El Harrach, Algiers, Algeria
  • Hakim Lounici Ecole Nationale Polytechnique, Unité URIE, 10 Avenue Pasteur, El Harrach, Algiers, Algeria

DOI:

https://doi.org/10.13171/mjc.3.1.2014.10.04.23

Abstract

The main purpose of this study is the use of TiO2 as catalyst in thin film fixed bed reactor (TFBR) for the treatment of landfill water with the high initial concentration of recalcitrant organic matter. The effectiveness treatment process was determined by the evaluation of the influence of the experimental parameters such as the pH on the Chemical Oxygen Demand (COD) and NH4+ concentration. The experimental assays were performed by varying the pH value from 5 to 6. The results obtained after treatment using this process was relevant. Indeed, a decrease of about 92% of the COD was achieved at pH maintained at 5. Moreover, the value of the BOD5/COD ratio obtained indicated that the water obtained after treatment are favorable for biological treatment. However, the NH4+ concentration was not affected by this process and remained at its high value.

References

- T. A. Kurniawan, W. Lo, G. YS Chan, Chemical Engineering Journal, 2006. 125, 35-57.

- P. B. Moraes, R. Bertazzoli , Chemosphere, 2005, 58, 41-46.

- S. Renou, J. G. Givaudan, S. Poulain, F. Dirassouyan, P. Moulin, Journal of Hazardous Materials, 2008, 150, 468-493.

-Y. Deng, J. D. Englehardt, Waste Management, 2007, 27, 380-388.

-T. A. Kurniawan, Journal of Hazardous Materials, 2006, 129, 80-100.

-J. R. Banu, S. Anandan, S. Kaliappan, I-T.Yeom, Solar Energy, 2008, 82, 812-819.

-P. Bouras, P. Lianos, Catalysis Letters, 2008, 123, 220-225.

-I. Arslan, I.A. Balcioglu, D.W. Bahnemann, Applied Catalysis B : Environmental, 2000, 26, 193-206.

- R. Dillert, U. Siemon, D. Bahnemann, Chemical Engineering & Technology, 1998, 21, 356-358.

- D. Gumy, A. Rincon, R. Hajdu. C. Pulgarin, Solar Energy, 2006, 80, 1376-1381.

- R. Dillert, S. Vollmer, M. Schober, J. Theurich, D. Bahnemann, H-J.Arntz, K. Pahlmann, J. Wienefeld, T. Schmedding, G. Sager, Chemical Engineering & Technology, 1999, 22, 931-934.

- S. Adjimi, N. Sergent, J.-C.Roux, F. Delpech, M. PeraTitus, K. Chhor, A. Kanaev, P.-X.Thivel, 2014, Applied Catalysis B, Environmental, http://dx.doi.org/10.1016/j.apcatb.2014.02.011

- J. Mo, Y. Zhang, Q. Xu, J. Joaquin Lamson, R. Zhao, Atmospheric Environment, 2009, 43, 2229-2246

- P. Pichat, Self-Cleaning Materials Based on Solar Photocatalysis.In. New and Future Developments in Catalysis: Solar Photocatalysis, 2013, 167-190

- Z. Huang, P.C. Maness, D.M. Blake, E.J. Wolfrum, S.L Smolinski. W.A. Jacoby, Journal of Photochemistry and Photobiology A: Chemistry, 2000, 130, 163-170.

- M. Faure, F. Gerardin, J.C. Andre, M.N. Pons, O. Zahraa, Journal Of Photochemistry and Photobiology A-Chemistry, 2011, 222, 323-329.

- B. Trouiller, R. Reliene, A. Westbrook, P. Solaimani, R.H Schiestl, Cancer Research, 2009, 69, 8784-8789

- A. Vaseashta, In Water Treatment Technologies for the Removal of High-Toxity Pollutants; ed. by M. Václavíková, K. Vitale, G.P. Gallios, L. IvaniÄová; Springer, 2010, pp. 1-16

- W.Z. Tang, Physicochemical treatment of hazardous wastes, CRC Press LLC, 2004.

- J. Hagen, Industrial Catalysis: A Practical Approach, Wiley-VCH, 2006.

– M. Kaneko, I. Okuro, Photocatalysis: Science and Technology, Springer, 2002.

- R. Pelton, X. Geng, M. Brook, Advances In Colloid and Interface Science, 2006, 127, 43-53.

- P. Escaffre, P. Girard, J. Dussaud, L. Bouvier, U.S. patent PCT FR99 007 48,1999.

- C. Guillard, J. Disdier, C. Monnet, J. Dussaud, S. Malato, J. Blanco, M. I. Maldonado, J.-M. Herrmann, Applied Catalysis B-Environmental 2003, 46, 319-332.

- Standard Methods for Examination of Water and Wastewater, 20th ed.,American Public Health Association, American Water Works Association,Water Pollution Federation, Washington DC, USA, 1999.

- M. Bodzek, J. Surmacz-Gorska, Y.T Hung, In Handbook of Industrial and Hazardous Wastes Treatment; ed by K. Lawrence, Y.T.H. Wang, H.L. Howard; Marcel Dekker, Inc., New York, USA, 2004, pp. 1150-1204.

- R. Chemlal, N. Abdi, N. Drouiche, H. Lounici, A. Pauss, N. Mameri, Ecological Engineering, 2013, 51, 244-248

- P. Flyhammar, Journal of Environmental Quality, 1995, 24, 612-619.

- B. Bayarri, J. Giménez, D. Curco, S. Esplugas, Catalysis Today, 2005, 101, 227-236.

- S. Liu, M. Lim, R. Fabris, C. Chow, K. Chiang, M. Drikas, R. Amal, Chemosphere, 2008, 72, 263-271.

- M. Cho, H. Chung, W. Choi, J. Yoon, Applied And Environmental Microbiology, 2005, 71, 270-275.

- T. Oppenländer, Photochemical Purification of Water and Air, WILEY-VCH, Weinheim, 2003.

- T. M. El-Morsi, W. R Budakowski, A. S. Abd-El-Aziz, K. J Friesen, Environmental Science & Technology, 2000, 34,1018-1022.

- M. R. Hoffmann, ST. Martin, W. Choi, DW. Bahnemman, Chemical Reviews, 1995,95, 69-96.

- B. Bayarri, J. Giménez, D. Curco, S. Esplugas, Catalysis Today, 2005, 101, 227-236.

- M.R. Hoffmann, S.T. Martin, W. Choi, D.W. Bahnemman, Chemical Reviews, 1995, 95, 69-96

- S.P. Cho, S.C. Hong, S. Hong, Applied Catalysis B : Environmental, 2002, 39, 125-133.

Downloads

Published

2014-04-10

Issue

Section

Environmental Chemistry